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1Author    V. B. Ankova3, N. N. Ikolova3, M. M. ArcuccibRequires cookie*
 Title    A New Lignan from Brazilian Propolis  
 Abstract    The known flavonoid kaempferid 4 and a new benzofurane lignan 1 were isolated from Brazilian propolis. The new lignan is a suitable taxonomic marker and gives new possibilities for identification of propolis plant sources in the tropical regions. In tro d u ctio n 
  Reference    Z. Naturforsch. 51c, 735—737 (1996); received June 13/June 26 1996 
  Published    1996 
  Keywords    Propolis, Lignans, Flavonoids 
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 TEI-XML for    default:Reihe_C/51/ZNC-1996-51c-0735.pdf 
 Identifier    ZNC-1996-51c-0735 
 Volume    51 
2Author    W. Greenaway, T. Scaysbrook, F. R. WhatleyRequires cookie*
 Title    Composition of Propolis in Oxfordshire, U.K. and its Relation to Poplar Bud Exudate  
 Abstract    Propolis balsam from four locations in Oxfordshire was analysed. The balsam was qualitatively similar but showed large quantitative differences in composition. These quan-titative differences are related to the bud exudate composi-tion of the poplars from which balsam was gathered. 
  Reference    Z. Naturforsch. 43c, 301—305 (1988); received November 13 1987 
  Published    1988 
  Keywords    Propolis, Poplar Bud Exudate, Bees 
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 TEI-XML for    default:Reihe_C/43/ZNC-1988-43c-0301_n.pdf 
 Identifier    ZNC-1988-43c-0301_n 
 Volume    43 
3Author    G. Boudourova-Krasteva3, Vassya Bankova3, J. M. Sforcinb, N. Nikolova3, S. Popov3Requires cookie*
 Title    Phenolics from Brazilian Propolis  
 Abstract    The main phenolic constituents from Brazilian propolis, originating from Sao Paulo State, were isolated and identified: three flavonoids, a prenylated coumaric acid and two new benzopyranes, E and Z 2,2-dimethyl-6-carboxyethenyl-8-prenyl-2H-benzopyranes. 
  Reference    Z. Naturforsch. 52c, 676—679 (1997); received April 7/June 9 1997 
  Published    1997 
  Keywords    Propolis, Phenolics, Flavonoids, Benzopyranes 
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 TEI-XML for    default:Reihe_C/52/ZNC-1997-52c-0676.pdf 
 Identifier    ZNC-1997-52c-0676 
 Volume    52 
4Author    Z. NaturforschRequires cookie*
 Title      
 Abstract    Three samples of Brazilian geopropolis, collected by three indigenous bee species, were investigated by GC/MS. More than 50 compounds were identified, mainly terpenoids and phenolics. The chemical composition of propolis gathered by different bee species was dif­ ferent. 
  Reference    Z. Naturforsch. 53c, 402 (1998); received February 11/March 24 1998 
  Published    1998 
  Keywords    Geopropolis, Propolis, Polyphenols, Terpenoids 
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 TEI-XML for    default:Reihe_C/53/ZNC-1998-53c-0402.pdf 
 Identifier    ZNC-1998-53c-0402 
 Volume    53 
5Author    Milena Velikova3, Vassya Bankova, Kadriye Sorkunb, Saadi Houcinec, Iva Tsvetkovad, A. KujumgievdRequires cookie*
 Title    Propolis from the Mediterranean Region: Chemical Composition and Antimicrobial Activity  
 Abstract    The chemical composition of propolis from Bulgaria, Turkey, Greece and Algeria was investigated by GC-MS. All of them contained mainly flavonoids and esters of caffeic and ferulic acids, which indicated that their main source are buds of poplars of the taxonomic section Aegieros. Some Turkish samples contained a low percent of diterpenic acids, while in Algerian samples significant amounts of a hydroxyditerpenic acid (M=322, its structure not determined by its MS) were found. All samples showed significant antibacterial and weak to moderate antifungal activity. 
  Reference    Z. Naturforsch. 55c, 790—793 (2000); received May 10/June 19 2000 
  Published    2000 
  Keywords    Propolis, Populus, Antimicrobial Activity 
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 TEI-XML for    default:Reihe_C/55/ZNC-2000-55c-0790.pdf 
 Identifier    ZNC-2000-55c-0790 
 Volume    55 
6Author    Ahm Ed, G. Hegazi, FatenK. Abd, El HadyRequires cookie*
 Title    Egyptian Propolis: 1-Antimicrobial Activity and Chemical Composition of Upper Egypt Propolis  
 Abstract    The antimicrobial activity of four propolis samples collected from Upper Egypt against Staphylococcus aureus; Escherichia coli and Candida albicans was evaluated. There was a variation in the antimicrobial activity according to the propolis origin. Banisweif propolis showed the highest antimicrobial activity against Staphylococcus aureus, Escherichia coli and Candida albicans, but Fayoum propolis had moderate activity against all tested pathogens. Propolis collected from Assiut and Souhag gave lower antimicrobial activity. Propolis samples were investigated by GC/MS, 71 compounds were identified, 14 being new for propolis. Banisweif propolis is characterized by the presence of 7 caffeate esters and 4 triterpenoids. Fayoum propolis showed the highest amount of lactic acid and the presence of 3 chalcones. But Assiut propolis is characterized by the presence of 4 prenylated coumar-ates. Souhag propolis is characterized by the presence of 5 aliphatic dicarboxylic acids and some other new compounds to propolis. 
  Reference    Z. Naturforsch. 56c, 82—88 (2001); received July 24/October 9 2000 
  Published    2001 
  Keywords    Propolis, Polyphenols, Antimicrobial Activity 
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 TEI-XML for    default:Reihe_C/56/ZNC-2001-56c-0082.pdf 
 Identifier    ZNC-2001-56c-0082 
 Volume    56 
7Author    O. Rlando, M. Uñoz3, RaúlC. Peñab, Enrique Ureta, GloriaM. Ontenegro0, B. Arbara, N. TimmermanncRequires cookie*
 Title    Propolis from Chilean Matorral Hives  
 Abstract    Viscidone (0.5%), vanillin, 3',4'-(m ethylendioxy)acetophenone, 3-ethoxy-4-methoxybenz-aldehyde, cinnamic acid, 3-methoxy-4-hydroxymethyl ester were isolated from propolis o f hives from Cuncumen. This is the first report on propolis composition o f an arid and a Mediterranean type climate area. 
  Reference    Z. Naturforsch. 56c, 269 (2001); received September 8/N ovem ber 16 2000 
  Published    2001 
  Keywords    Propolis, Structure Elucidation, Plant Sources 
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 TEI-XML for    default:Reihe_C/56/ZNC-2001-56c-0269.pdf 
 Identifier    ZNC-2001-56c-0269 
 Volume    56 
8Author    Milena Popova3, Vassya Bankova3, Iva Tsvetkovab, Christo Naydenskib, MarioVides SilvacRequires cookie*
 Title    The First Glycosides Isolated from Propolis: Diterpene Rhamnosides  
 Abstract    Two diterpene glycosides, e«r-S(17)-labden-15-0-a-L-rhamnoside and e«r-8(17)-labden-15-0-(3'-0-acetyl)-a-L-rham noside (new natural compounds) were isolated from propolis from El Salvador. The compounds showed significant antibacterial activity and moderate toxicity to Artemia salina nauplii. These are the first glycosides reported in bee glue. 
  Reference    Z. Naturforsch. 56c, 1108—1111 (2001); received July 19/August 23 2001 
  Published    2001 
  Keywords    Propolis, Labdane Glycosides, Antibacterial Activity 
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 TEI-XML for    default:Reihe_C/56/ZNC-2001-56c-1108.pdf 
 Identifier    ZNC-2001-56c-1108 
 Volume    56 
9Author    Nevin Keskin3, Selçuk Hazir3, K. Hüsnü, Can Baserb, Mine KürkçüoglubRequires cookie*
 Title    Antibacterial Activity and Chemical Composition of Turkish Propolis  
 Abstract    The antibacterial activities of propolis samples have been examined in vitro, according to the principles accepted for the determination of a similar activity of antibiotics with the use of solid and liquid media. It has been found that propolis extracts showed antibacterial activ­ ity through a range of commonly encountered gram positive cocci (5. aureus, beta hem. Streptococus), but had weak activity against gram negative bacteria (E . coli, P. aeruginosa). GC/MS analysis showed that propolis samples contain a variety of chemical compounds in­ cluding aromatic compounds, fatty acid esters and sesquiterpenes. 
  Reference    Z. Naturforsch. 56c, 1112—1115 (2001); received May 4/August 23 2001 
  Published    2001 
  Keywords    Propolis, Hive Product, Antibacterial Agent 
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 TEI-XML for    default:Reihe_C/56/ZNC-2001-56c-1112.pdf 
 Identifier    ZNC-2001-56c-1112 
 Volume    56 
10Author    Requires cookie*
 Title    A Novel Caffeic Acid Derivative and Other Constituents of Populus Bud Excretion and Propolis (Bee-Glue)  
 Abstract    E ck h a rd W ollenw eber, Y oshinori A sakaw a*, D etlef Schillo, U lrich L eh m an n , and H eid ru n W eigel The bud exudates of Populus nigra, P. trichocarpa, and P. grandidentata x tremuloides were analyzed for the presence of phenolics and flavonoids. A novel natural product, caffeic acid y.y-dimethylallyl ester, was identified from P. nigra, along with further phenolics such as /?-hydroxy-acetophenone, dimethyl caffeic acid, cinnamoyl cinnamata and vanillin. The flavonoid aglycones correspond to those reported earlier. Propolis samples from the Sonoran Desert were shown to exhibit the flavonoid pattern that is typical for poplar bud exudates, thus confirming this material as the major source for bee-glue. Only a single flavonoid might originate from the leaf exudate of a desert shrub. 
  Reference    Z. Naturforsch. 42c, 1030—1034 (1987); received May 8/May 21 1987 
  Published    1987 
  Keywords    Populus (Salicaceae), Bud Exudate, Propolis, Phenolics, Flavonoids 
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 TEI-XML for    default:Reihe_C/42/ZNC-1987-42c-1030.pdf 
 Identifier    ZNC-1987-42c-1030 
 Volume    42 
11Author    T. Hashimoto, M. Tori, Y. Asakawa, E. WollenweberRequires cookie*
 Title    Synthesis of Two Allergenic Constituents of Propolis and Poplar Bud Excretion  
 Abstract    The prenyl ester and the phenylethyl ester of caffeic acid, formed in the bud excretion of poplar species, were shown recently to be the major contact allergens in bee-glue. An unambiguous synthesis of these compounds, based on the reaction of caffeic acid with l-bromo-3-methyl-2-butene and with ß-bromoethylbenzene, respectively, is reported. The synthetic products confirm the previously described structures of the natural products and allow further testing of their allergenic properties. 
  Reference    Z. Naturforsch. 43c, 470—472 (1988); received January 25 1988 
  Published    1988 
  Keywords    Propolis, Contact Allergens, Prenyl Caffeate, Phenylethyl Caffeate, Synthesis 
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 TEI-XML for    default:Reihe_C/43/ZNC-1988-43c-0470_n.pdf 
 Identifier    ZNC-1988-43c-0470_n 
 Volume    43 
12Author    S. Scheller, M. Czauderna, W. Krol, J Z Konecki+, Czuba, J. Gabrys+, M. Glowacka+, J. Shani+Requires cookie*
 Title    Trace Elements in Propolis and in its Ethanolic Extract (E E P ) as Determined by Neutron Activation Analysis  
 Abstract    Propolis is a natural composite balsam, manufactured by honey bees, and active biochemically. Some of its biologi­ cal effects are attributed to its ability to stimulate enzymatic systems, which in many instances involve trace elements. In the present study we assayed propolis and its ethanolic ex­ tract (EEP) for trace elements, and quantified them with the aid of neutron activation analysis. Four elements that have been detected in propolis and EEP for the first time are Na. Cr, Co (ppm) and Ag (ppb). The wide concentra­ tion range of the inorganic components in various batches of propolis and EEP is due to the difference in their extrac­ tion capacities, and to the variability in the environmental pollutants and the flora at the beehive sites. 
  Reference    Z. Naturforsch. 44c, 170—172 (1989); received September 28 1988 
  Published    1989 
  Keywords    Propolis, Trace Elements, Neutron Activation Honey Bee 
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 TEI-XML for    default:Reihe_C/44/ZNC-1989-44c-0170_n.pdf 
 Identifier    ZNC-1989-44c-0170_n 
 Volume    44 
13Author    Regina Volpert, ErichF. ElstnerRequires cookie*
 Title    Biochemical Activities of Propolis Extracts I. Standardization and Antioxidative Properties of Ethanolic and Aqueous Derivatives  
 Abstract    Ethanolic extracts of Propolis are used as antiinflammatory and wound healing drugs since ancient times. In order to facilitate a comparison of different extracts, the standardization on the basis of quantitative determination of prominent components of these extracts has been substituted for simple biochemical "activity" tests. One of these activity tests bases on the in­ hibition of peroxidase-catalyzed oxidation of indole acetic acid indicating the presence of a defined mixture of monophenolic and diphenolic compounds. Other tests (diaphorase-cata-lyzed reductions and xanthine oxidase-catalyzed oxidations) demonstrate significant radical scavenging properties. Water-soluble extracts of propolis exhibit higher antioxidative and inhibitory activities as compared to the ethanolic extract. 
  Reference    Z. Naturforsch. 48c, 851—857 (1993); received June 21/August 161993 
  Published    1993 
  Keywords    Propolis, Peroxidase, Xanthine Oxidase, Diaphorase, Indole Acetic Acid Oxidation 
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 TEI-XML for    default:Reihe_C/48/ZNC-1993-48c-0851.pdf 
 Identifier    ZNC-1993-48c-0851 
 Volume    48 
14Author    Josep Serra Bonvehf, FrancescVentura CollRequires cookie*
 Title    Phenolic Composition of Propolis from China and from South America  
 Abstract    Flavonoids and other phenolic compounds were determined in 15 samples of propolis originating from China, from Brazil, and from Uruguay. A total of 24 compounds were identified using mainly HPLC and a few other analytical methods. The most abundant com­ pounds found were benzoic acid and benzaldehyde derivatives, flavones, flavonols. and flava-nones. 80% of the samples contained at least 22 g/100 g of flavonoids, primarily acacetin, isorhamnetin, apigenin, and pinocembrin. The flavonoid patterns were sufficiently distinctive to permit discrimination between propolis from China, from Uruguay, and from Brazil. 
  Reference    Z. Naturforsch. 49c, 712 (1994); received March 18/August 9 1994 
  Published    1994 
  Keywords    Propolis, China, South America, Phenolic Constituents, Flavonoids 
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 TEI-XML for    default:Reihe_C/49/ZNC-1994-49c-0712.pdf 
 Identifier    ZNC-1994-49c-0712 
 Volume    49 
15Author    V. Bankova3, R. Christov3, A. Kujumgievb, M. C. Marcuccic, S. Popov3Requires cookie*
 Title    Chemical Composition and Antibacterial Activity of Brazilian Propolis  
 Abstract    Four samples of Brazilian propolis were investigated by GC/MS of different fractions. 32 volatile compounds, (10 of them new for propolis), as well as 12 more polar compounds (one of them new for propolis) were identified. Antibacterial activity was found in some propolis fractions. 
  Reference    Z. Naturforsch. 50c, 167 (1995); received January 10/January 20 1995 
  Published    1995 
  Keywords    Propolis, Polyphenols, Volatiles, GC/MS, Antibacterial Activity 
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 TEI-XML for    default:Reihe_C/50/ZNC-1995-50c-0167.pdf 
 Identifier    ZNC-1995-50c-0167 
 Volume    50 
16Author    V. Bankova3, M. C. Marcuccib, S. Simova3, N. Nikolova3, A. Kujumgievc, S. Popov3Requires cookie*
 Title    Antibacterial Diterpenic Acids from Brazilian Propolis  
 Abstract    Four labdane-type diterpenic acids and syringaldehyde were isolated and identified from Brazilian propolis. A ll the com pounds exhibit antibacterial activity. The diterpenes, found for the first time in propolis, are typical for som e Araucaria species and thus indicate a possible plant source of Brazilian propolis. 
  Reference    Z. Naturforsch. 51c, 277 (1996); received Novem ber 23 1995/January 24 1996 
  Published    1996 
  Keywords    Propolis, Diterpenic Acids, Antibacterial Activity, Propolis Plant Sources 
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 TEI-XML for    default:Reihe_C/51/ZNC-1996-51c-0277.pdf 
 Identifier    ZNC-1996-51c-0277 
 Volume    51 
17Author    Purusotam Basnet3, TetsuyaM. Atsunob, Richard Neidlein3Requires cookie*
 Title    Potent Free Radical Scavenging Activity of Propol Isolated from Brazilian Propolis  
 Abstract    We evaluated free radical scavenging activity of the water, methanol and chloroform ex­ tracts of propolis in l,l-diphenyl-2-picrylhydrazyl (DPPH) free radical and xanthine-xanthine oxidase (XO D) generated superoxide anion assay systems. The free radical scavenging activ­ ity guided fractionation and chemical analysis led to the isolation of a new compound, propol {3-[4-hydroxy-3-(3-oxo-but-l-enyl)-phenyl]-acrylic acid) from the water extract, which was more potent than most common antioxidants such as vitamin C and vitamin E (a-tocopherol) in these assay systems. 
  Reference    Z. Naturforsch. 52c, 828—833 (1997); received August 7/September 19 1997 
  Published    1997 
  Keywords    Propol, Propolis, Free Radicals, Superoxide Anion, Antioxidative Activity 
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 TEI-XML for    default:Reihe_C/52/ZNC-1997-52c-0828.pdf 
 Identifier    ZNC-1997-52c-0828 
 Volume    52 
18Author    M. C. Marcucci3, Jose Rodriguez, F. Ferreresc, V. B. An K O V, Robson Groto6, S. PopovdRequires cookie*
 Title    Chemical Composition of Brazilian Propolis from Sao Paulo State  
 Abstract    Two propolis samples from Sao Paulo State were investigated by GC/MS. 39 compounds were identified, 8 being new for propolis. Both samples showed some similarities in their qualitative composition. In one of them, coum aric acid and its prenylated derivatives predo­ minated, while in the other one triterpenic alcolhols were the main constituents. 
  Reference    Z. Naturforsch. 53c, 117 (1998); received O ctober 7/D ecem ber 8 1997 
  Published    1998 
  Keywords    Propolis, GC/MS, Phenolic Acids, Triterpenes 
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 TEI-XML for    default:Reihe_C/53/ZNC-1998-53c-0117.pdf 
 Identifier    ZNC-1998-53c-0117 
 Volume    53 
19Author    TetsuyaM. Atsuno3, Masahiro Saitob, YasuyukiM. Atsumotob, JunjiM. OrikawabRequires cookie*
 Title    A New Benzo-y-pyran Derivative Isolated from Propolis  
 Abstract    The methanol extract of Brazilian propolis was fractionated by HPLC, based on human hepatocellular carcinoma (HuH 13) cell cytotoxicity assay. A new benzo-y-pyran derivative (PM-3) with a molecular formula of Q 9 H 2 2 O3 (MW: 298.38) was isolated. The structure of this colorless compound was determined as 3-[2-dimethyl-8-(3-methyl-2-butenyl) benzopy-ran]-6 -propenoic acid. This compound was chemically synthesized by cyclisation of artepillin C (3-[4-hydroxy-3,5-bis (3-methyl-2-butenyl) phenyl]-2-propenoic acid). 
  Reference    Z. Naturforsch. 53c, 1037—1039 (1998); received July 15/September 14 1998 
  Published    1998 
  Keywords    Propolis, Benzopyran Derivative, Artepillin C, Cytotoxicity 
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 TEI-XML for    default:Reihe_C/53/ZNC-1998-53c-1037.pdf 
 Identifier    ZNC-1998-53c-1037 
 Volume    53 
20Author    WalterA. Bretz3, D. J. Chiego, M. C. Marcucci0, I. Cunhad, A. Custódiod, L. G. Schneider3Requires cookie*
 Title    Preliminary Report on the Effects of Propolis on Wound Healing in the Dental Pulp  
 Abstract    The purpose of this investigation was to determ ine the antimicrobial and healing potential of propolis on direct dental pulp exposures. This study used 25 adult male rats. Pulp expo­ sures were perform ed and animals were allocated to propolis and calcium hydroxide (C a(O H) 2 groups. Animals were killed on days 5, 7, 10, and 14. The teeth were routinely processed for histological evaluation. N on-param etric tests were employed to analyze the data. No significant differences were found between study groups on the wound healing of the dental pulp. Both substances were com parable in exhibiting normal reorganization of the pulp and no increased vascularity, and were equally efficacious in maintaining a low inflam­ matory and microbial cell population as well as in stimulating the formation of reparative dentin. 
  Reference    Z. Naturforsch. 53c, 1045—1048 (1998); received May 29/August 3 1998 
  Published    1998 
  Keywords    Propolis, Dental Pulp, Wound Healing, Antimicrobial 
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 TEI-XML for    default:Reihe_C/53/ZNC-1998-53c-1045.pdf 
 Identifier    ZNC-1998-53c-1045 
 Volume    53 
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